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FIG. 2. The deleterious effect of plasma self-emission on the diagnostics is avoided by a frequency shift in the probe beam and aggressive optical filtering. (a) Near the critical surface of laser-plasma interaction, plasma selfemission at 400 nm saturates imagery. (b) To avoid this effect, the probe beam is frequency shifted to 840 nm, amplified, then frequency doubled to 420 nm. At the imaging cameras, notch filters are used to remove plasma self-emission at the pump’s second harmonic, 400 nm. The notch filter transmission band includes the entire probe beam spectrum and only the tail of the plasma selfemission spectrum. (c) The effect of the frequency shift and optical notch filters is to reveal previously obscured interaction areas.

is the source of the plasma self-emission that is the subject of this subsection. Plasma self-emission complicates and frustrates probe-beam interferometry and shadowgraphy because it obscures areas of interest near the critical surface (see Fig. 2(a)). The solution to this obfuscation problem, which we have implemented in this setup, is to apply optical filtering that excludes plasma self-emission while passing the probe beam. Even with specially selected optical notch filters, this is only possible if the probe spectrum sits outside of the plasma selfemission spectrum. However, because the pump and probe share a common oscillator, the probe pulse naturally shares the frequency of the pump harmonic. To circumvent this issue, the frequency of the probe pulse is shifted in two steps.

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Prior to amplification, the broadband 800 nm seed pulse of the probe beam is optically filtered using Schott RG850 glass, moving the central wavelength to 840 nm by preferentially attenuating lower wavelengths. Next, a hard spectral cutoff is applied in the pulse stretcher, by physically clipping lower wavelength regions of the beam during grating dispersion. This frequency-shifted (and much attenuated) pulse is next passed through a regenerative amplifier, which smooths the spectral profile, and after re-compression the pulse remains centered at 840 nm. Finally, the probe beam is frequency doubled to 420 nm via a β-barium borate crystal (AR/AR coated, 300 μm thick, Type I). During imaging, two optical notch filters (Semrock FF01-420/10-25; 10 nm bandwidth, and nominally 15 nm FWHM) select for the 420 nm probe and reject the plasma self-emission at 400 nm (Figs. 2(b) and 2(c)).

V. ACQUISITIONS AND ANALYSIS

By varying probe beam delay time, an image sequence can be created that shows the development of pre-plasma, the main ultra-intense pulse interaction, and the hydrodynamic recovery of the target (see Fig. 3). The image acquisitions are performed in the following way. A sequence of delay times is chosen so as to acquire many frames shortly before the main pulse interaction while keeping a wide temporal view of the interaction. Once programmed, the sequence is serially executed. To create a given delay, Pockels cell seed selection and delay line position are adjusted automatically. For each delay, one shadowgraphic frame and three interferometric frames are acquired (corresponding to three positions of the piezoelectric mirror which varies Michelson interferometer phase difference). Because stochastic events can cause occasional extreme outliers shot-to-shot, 10 images are acquired for each frame, corresponding to ten independent laser shots. The image most similar to the average is incorporated as the frame. Interferograms must be analyzed to recover phase data. Phase shifts are reconstructed from fringe shifts using the

FIG. 3. Precise probe pulse timing (< 40 fs resolution) over a wide dynamic range (> 10 μs) gives a detailed view of pre-plasma evolution, intense laser-plasma interaction, and target recovery. Upper sequence: Recovered phase shifts from interferometry show the in-vacuum development of pre-plasma nanoseconds before the main interaction, consistent with known pre-pulse on this timescale. Delay times relative to the main ultra-intense laser pulse are marked. Interferometric reconstruction after the main pulse arrives (≥ 0 fs, not shown) fails due to steep phase gradients. Lower sequence: Shadowgraphy shows timescales of in-air target evolution: hydrodynamic reaction in picoseconds, expansion in nanoseconds, and recovery in microseconds.

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FIG. 4. To aid in the reconstruction of phase dependent imagery from fringe shifts, three separate 120◦ phase-shifted (temporally sheared) interferograms are acquired for each probe delay. Left: an interferogram is shown for −15 ps delay for an in-vacuum target. Its corresponding phase image is reconstructed using the Speckle Phase of Difference algorithm in IDEA software – the vertical dashed line represents the rightmost boundary of reliable phase reconstruction. Abel inversion allows recovery of index of refraction and potentially electron density. Right: recovered index of refraction shifts for the interferogram at left are shown. The radial index change from negative to positive suggests pre-plasma on-axis and ablated neutral material off-axis.

IDEA software16 Speckle Phase of Difference algorithm (three-frame technique, 120◦ phase shift). Abel inversion can be performed to recover the changes in index of refraction (see Fig. 4 for an experimental example). Abel inversion analysis requires an added assumption of the experiment’s radial symmetry, about the laser axis. From the Abel inversion, electron densities can potentially be inferred. VI. SUMMARY AND CONCLUSIONS

We have described a frequency-shifted, femtosecondgated interferometric setup and demonstrated its capability for a flowing water jet experiment in which this target is irradiated by nanosecond-scale and picosecond-scale pre-pulses in advance of the arrival of an ultra-intense (1018 W/cm2 ) pulse. The combination of a timing system for observing evolution from femtoseconds to microseconds and elimination of plasma self-emission noise light delivers improved shadowgraphy and interferometry. Phase shift reconstruction from interferometry reveals changes in the index of refraction near the target. This information can be used to infer electron densities through Abel inversion. With precise optical filtering and by frequency shifting the probe pulse away from the selfemission frequencies, the problem of plasma self-emission is avoided. The diagnostic has been demonstrated to produce interferometric and shadowgraphic image sequences of lasermatter interactions which show nanosecond formation of preplasma, femtosecond interaction of the ultra-intense main pulse, picosecond hydrodynamic expansion, and microsecond recovery of the target. Fielding the diagnostic has already contributed in two ways to our experimental understanding. First, tens-of-microseconds target recovery time indicates that the experiment could be performed at significantly higher than

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kHz repetition rates. Second, expectations prior to the arrival of the main pulse of pre-plasma formation along the laser axis with neutral material off-axis are confirmed. By providing on-demand femtosecond resolution at arbitrary delay times, this diagnostic will soon be used to track the effects of known femtosecond-duration pre-pulses as they arrive on target picoseconds to nanoseconds prior to the main pulse, and to improve laser-driven electron acceleration and X-ray production techniques.17 Future improvements to the diagnostic may include additional views of the interaction region or on-the-fly interferogram analysis for fast feedback to the experimenter. ACKNOWLEDGMENTS

This research was sponsored by the Quantum and NonEquilibrium Processes Department of the (U.S.) Air Force Office of Scientific Research (USAFOSR), under the management of Dr. Enrique Parra, Program Manager. S.F. was supported in part by the DOD HPCMP high performance computing internship program. The authors thank Mario Manuel, University of Michigan, for insightful discussions. 1 T. Hosokai, K. Kinoshita, A. Zhidkov, K. Nakamura, T. Watanabe, T. Ueda,

H. Kotaki, M. Kando, K. Nakajima, and M. Uesaka, Phys. Rev. E 67, 036407 (2003). 2 M. Kaluza, J. Schreiber, M. I. K. Santala, G. D. Tsakiris, K. Eidmann, J. Meyer-ter Vehn, and K. J. Witte, Phys. Rev. Lett. 93, 045003 (2004). 3 K.-H. Hong, B. Hou, J. A. Nees, E. Power, and G. A. Mourou, Appl. Phys. B 81, 447 (2005). 4 C. Orban, M. Fatenejad, S. Chawla, S. C. Wilks, and D. Q. Lamb, e-print arXiv:1306.1584 [physics]. 5 F. Dollar, P. Cummings, V. Chvykov, L. Willingale, M. Vargas, V. Yanovsky, C. Zulick, A. Maksimchuk, A. G. R. Thomas, and K. Krushelnick, Phys. Rev. Lett. 110, 175002 (2013). 6 I. H. Hutchinson, Principles of Plasma Diagnostics (Cambridge University Press, 2005). 7 Z. Wu, X. Zhu, and N. Zhang, J. Appl. Phys. 109, 053113 (2011). 8 V. V. Temnov, K. Sokolowski-Tinten, P. Zhou, and D. v. d. Linde, Appl. Phys. A 78, 483 (2004). 9 S. Le Pape, Y. Y. Tsui, A. Macphee, D. Hey, P. Patel, A. Mackinnon, M. Key, M. Wei, T. Ma, F. N. Beg, R. Stephens, K. Akli, T. Link, L. VanWoerkom, and R. R. Freeman, Opt. Lett. 34, 2997 (2009). 10 P. McKenna, D. Carroll, O. Lundh, F. Nürnberg, K. Markey, S. Bandyopadhyay, D. Batani, R. Evans, R. Jafer, S. Kar, D. Neely, D. Pepler, M. Quinn, R. Redaelli, M. Roth, C.-G. Wahlström, X. Yuan, and M. Zepf, Laser Part. Beams 26, 591 (2008). 11 J. Uhlig, C.-G. Wahlström, M. Walczak, V. Sundström, and W. Fullagar, Laser Part. Beams 29, 415 (2011). 12 W. Fullagar, M. Harbst, S. Canton, J. Uhlig, M. Walczak, C.-G. Wahlström, and V. Sundström, Rev. Sci. Instrum. 78, 115105 (2007). 13 Y. Y. Hung, Opt. Commun. 11, 132 (1974). 14 S. A. Crooker, F. D. Betz, J. Levy, and D. D. Awschalom, Rev. Sci. Instrum. 67, 2068 (1996). 15 D. von der Linde, H. Schulz, T. Engers, and H. Schuler, IEEE J. Quantum Electron. 28, 2388 (1992). 16 M. Hipp, J. Woisetschläger, P. Reiterer, and T. Neger, Measurement 36, 53 (2004). 17 C. Orban, J. T. Morrison, E. D. Chowdhury, J. A. Nees, K. Frische, and W. M. Roquemore, e-print arXiv:1405.6313 [physics].

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Parallax diagnostics of radiation source geometric dilution for iron opacity experimentsa) T. Nagayama, J. E. Bailey, G. Loisel, G. A. Rochau, and R. E. Falcon Sandia National Laboratories, Albuquerque, New Mexico 87185, USA

(Presented 2 June 2014; received 2 June 2014; accepted 27 June 2014; published online 17 July 2014) Experimental tests are in progress to evaluate the accuracy of the modeled iron opacity at solar interior conditions [J. E. Bailey et al., Phys. Plasmas 16, 058101 (2009)]. The iron sample is placed on top of the Sandia National Laboratories z-pinch dynamic hohlraum (ZPDH) radiation source. The samples are heated to 150–200 eV electron temperatures and 7× 1021 –4× 1022 cm−3 electron densities by the ZPDH radiation and backlit at its stagnation [T. Nagayama et al., Phys. Plasmas 21, 056502 (2014)]. The backlighter attenuated by the heated sample plasma is measured by four spectrometers along ±9◦ with respect to the z-pinch axis to infer the sample iron opacity. Here, we describe measurements of the source-to-sample distance that exploit the parallax of spectrometers that view the half-moonshaped sample from ±9◦ . The measured sample temperature decreases with increased source-tosample distance. This distance must be taken into account for understanding the sample heating. © 2014 AIP Publishing LLC. [http://dx.doi.org/10.1063/1.4889776] I. INTRODUCTION

Opacity quantifies photon absorption in matter and plays a crucial role in many high energy density plasmas, including inertial fusion plasmas and stellar interiors.1 Modeling opacities of ions with multiple bound electrons is very challenging and employs approximations that need to be experimentally validated.2, 3 Performing reliable opacity experiments is also challenging and must satisfy many criteria.2, 3 Measuring opacity becomes more difficult at higher temperature because the opacity sample has to be heated to the high temperature without significant gradients and has to be backlit by a bright radiation to minimize the effect of the hot sample plasma emission on the absorption measurement. The Sandia National Laboratories (SNL) Z machine (Z) provides a unique platform to perform opacity experiments at temperatures above 150 eV.4 The Z-pinch dynamic hohlraum (ZPDH) is a terawatt xray radiation source at Z that makes high-temperature opacity measurements possible.5 The opacity sample is located above the ZPDH radiation source and is radiatively heated. Most of the photons have energies above 600 eV. This powerful radiation streams through the sample and heats it without significant gradients.6 The ZPDH also provides a bright backlighter to mitigate the sample self-emission. Recently, we found that the opacity sample can reach higher temperatures and densities using the same radiation source only by changing the target configuration.6, 7 However, it was not clear why the change in the target configuration affects the sample temperature if the sample is heated by the same radiation source. To further optimize this high temperature opacity experimental platform, it is crucial to understand what dictates a) Contributed paper, published as part of the Proceedings of the 20th

Topical Conference on High-Temperature Plasma Diagnostics, Atlanta, Georgia, USA, June 2014.

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the sample temperature. In this article, we provide experimental evidence that the source-to-sample distance depends on the sample configuration. This distance controls the source geometric dilution at the sample, thereby affecting the sample temperature. II. SNL OPACITY EXPERIMENTS AND PARALLAX

The typical SNL opacity experimental setup is shown in Fig. 1. The target consists of a semi-circular FeMg sample sandwiched by a circular tamping material (e.g., plastic, CH), which we call a “half-moon” target. Mg is mixed in the Fe sample to diagnose the Fe conditions (i.e., electron temperature, Te , and electron density, ne ) using Mg K-shell spectroscopy.6, 8 This target is placed above the ZPDH radiation source, and the ZPDH radiation heats and backlights the sample.3, 5 The backlighter attenuated through the target is recorded by potassium acid phthalate crystal (KAP) spectrometers fielded along ±9◦ from the z-axis.8 An aperture above the target limits the spectrometers’ views to a 4 mm × 1 mm area. Each spectrometer has 4-6 slits, each 50 μm in width, at the halfway distance to the sample to provide spatial resolution of ∼0.1 mm along the aperture direction with a magnification of ∼1. The transmitted backlighter images are recorded on Kodak 2492 x-ray films with spatial and spectral resolution. Due to the finite source-to-sample distance, h, the spectrometer at +9◦ observes the backlighter bright spot through +9◦ , while the one at −9◦ the FeMg embedded side at xBL −9◦ observes it on the CH-only side at xBL (black dots in Fig. 1). This spectrometer configuration measures the FeMgattenuated and unattenuated spectra simultaneously, providing FeMg transmission spectra in a single experiment (shot). However, taking advantage of this parallax, we can also infer the backlighter location with respect to the “half-moon” +9◦ −9◦ and xBL as boundary (i.e., h and δ in Fig. 1) based on xBL

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FIG. 3. Backlighter images attenuated through the target recorded from −9◦ and +9◦ . FeMg is embedded at x > 0. Horizontal red solid and dashed lines indicate the locations of the “half-moon” boundary at x = 0 and the apparent −9◦ +9◦ backlighter peaks at x = xBL and x = xBL , respectively.

FIG. 1. Two space-resolving spectrometers located at ±9◦ with respect to the z-axis record the sample-transmitted backlighter images. Due to the angle difference, the spectrometers at ±9◦ ◦ see the ◦backlighter centered at different +9 −9 locations on the sample (i.e., xBL and xBL ). This parallax not only measures FeMg-attenuated and unattenuated spectra simultaneously, but it also characterizes the backlighter relative location with respect to the “half-moon” boundary, h and δ.

follows: ◦



−9  x +9 − xBL 1  +9◦ −9◦ h = BL , δ= x + xBL 2tan(9◦ ) 2 BL

(1)

assuming that the source-to-detector distance is much larger +9◦ −9◦ − xBL . than xBL +9◦ −9◦ and xBL from the data, one has to unTo extract xBL derstand the emergent intensity spatial profiles measured at ±9◦ (Fig. 2). The x-axis is defined such that the “half-moon” boundary is at x = 0 and the FeMg-embedded region is at x > 0. The hypothetical transmission spatial profile at a given wavelength (blue) is systematically lower at x > 0 due to the FeMg attenuation. The apparent backlighter spatial profiles (green) are centered at different locations with respect to the

FIG. 2. Idealized schematics illustrate how the backlighter (green) observed at different angles results in different emergent intensity spatial profiles (magenta).





+9 −9 sample for the ±9◦ spectrometers (i.e., xBL and xBL , respectively). While most of the backlighter spatial profile is attenuated through the FeMg region on the +9◦ spectrometer, only the backlighter wing is attenuated through FeMg on the −9◦ spectrometer. As a result, one expects to see a double peak in the emergent spatial profile at +9◦ , while one expects a skewed single peak at −9◦ . Figure 3 shows the data recorded by the spectrometers at ±9◦ . Each image is the average over four slit images to improve the signal-to-noise ratio and to average out random defects in the individual slit images.6 The horizontal (spectral) and vertical (spatial) axes are produced by the KAP crystals and the slits, respectively. The dark vertical lines correspond to Fe or Mg bound-bound absorption lines. The image recorded at +9◦ shows longer Fe and Mg lines than those recorded at −9◦ due to the apparent backlighter peak locations (Fig. 2). +9◦ −9◦ and xBL , one has to extract the In order to measure xBL locations of the “half-moon” boundary and the apparent backlighter peak. To objectively extract them, we take a spatial lineout on a strong bound-bound absorption line. The magenta curves in Fig. 4 show an example for the Mg Heα line (i.e., absorption due to 1s2 − 1s2p He-like Mg transition) at ∼9.17 Å (lineout λ = 0.02 Å). As discussed earlier, the magenta curve at +9◦ has a double peak, while the one at −9◦ has a skewed single peak. We approximate the spatial profile in the absence of the Mg Heα (green curves in Fig. 3) by averaging two spatial lineouts taken on each side of the Mg Heα line. The lineout locations for the +9◦ image are indicated by vertical green dashed lines in Fig. 3. The Heα line transmission is determined from the ratio of the magenta and green curves. The resultant transmission spatial profiles clearly show lowtransmission FeMg embedded regions, and the x-axis is defined from its inflection point. We note that the “half-moon” boundary is not as sharp as the one in Fig. 2. This is because of the instrument spatial resolution and the sample hydrody+9◦ namics integrated over the backlighter duration. Once xBL ◦ −9 and xBL are defined by the apparent backlighter peak locations on the defined x-axis, the backlighter location, h and δ, can be estimated from Eq. (1).

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FIG. 4. The spatial lineouts are extracted from Fig. 3 at Mg Heα (magenta) and its nearby continuum (green). Mg Heα bound-bound line transmission spatial lineouts (blue) are extracted by dividing the magenta by the green. The “half-moon” boundary and the x-axis are defined based on the transmission −9◦ +9◦ spatial lineouts, and xBL and xBL are defined based on the continuum peaks.

III. RESULTS

Parallax is systematically applied to ten Fe opacity shots performed under different sample configurations.6 There are three different CH configurations and multiple different Fe thicknesses for each configuration. There is one shot where the sample is raised by 1.5 mm from its nominal location. For each shot, parallax is applied to the available bound-bound lines that are strong enough to define the “half-moon” boundary from their line-transmission spatial profiles. The number of usable lines depends on their areal density, Stark line width, and the spectral range of the spectrometers used. For each shot, the mean h and its standard deviation are computed from parallax results of two to seven Fe and Mg lines. Parallax results from Fe and Mg lines agree with each other. The validity of this uncertainty estimate was also verified from the shots with four spectrometers, two each at +9◦ and −9◦ .

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Figure 5 summarizes the measured h as a function of Te inferred from Mg K-shell spectroscopy.6 We confirm a strong anti-correlation between h and Te (Pearson correlation coefficient = −0.91). To investigate this point synthetically, we use a 3D view factor code VISRAD9 and a calibrated ZPDH intensity image from one of our experiments to calculate the heating radiation at the sample as a function of the sample distance from the ZPDH radiation source. The details of the calculation will be discussed elsewhere. The blue curve in Fig. 5 shows the resultant radiation brightness temperature, TB , as a function of h. This result suggests that the radiation source heats the sample to different temperatures due to source radiation geometric dilution. The radiation brightness temperature is systematically higher than Te due to the complex heating mechanism involving radiation transport and hydrodynamics and beyond the scope of this article. Figure 5 also shows that, for similar Te , shot-to-shot variation in the inferred h is larger than the individual measurement uncertainties due to the 3D radiation transport effects of the backlighter. While Eq. (1) is derived assuming an instantaneous point backlighter, the actual backlighter emission is a result of the radiation transport through the 3D ZPDH plasma, which spatially varies over a few ns duration. Thus, the variation in the inferred h comes from the irreproducibility in the evolution of 3D ZPDH plasma and the resultant irreproducibility in the line-of-sight dependent effects on the measurements. We found that h was anti-correlated to Te and confirmed that the sample reached a different temperature due to the geometric dilution of the radiation source. The parallax results are important (i) to better understand our platform and further optimize SNL Z opacity experiments and (ii) to better understand the sample heating and accurately evaluate how close our sample is to local thermal equilibrium. ACKNOWLEDGMENTS

Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the (U.S.) Department of Energy (DOE) under Contract No. DE-AC0494AL85000. 1 D.

FIG. 5. There is a strong correlation between the measured electron temperature, Te , and the measured source-to-sample distance, h. The blue curve is a modeled radiation brightness temperature as a function of h.

Mihalas, Stellar Atmospheres, A Series of Books in Astronomy and Astrophysics, 2nd edition (W. H. Freeman, 1978). 2 T. Perry et al., Phys. Rev. E 54, 5617 (1996). 3 J. E. Bailey et al., Phys. Plasmas 16, 058101 (2009). 4 J. Bailey et al., Phys. Rev. Lett. 99, 265002 (2007). 5 G. A. Rochau et al., Phys. Plasmas 21, 056308 (2014). 6 T. Nagayama et al., Phys. Plasmas 21, 056502 (2014). 7 T. J. Nash et al., Rev. Sci. Instrum. 81, 10E518 (2010). 8 J. E. Bailey et al., Rev. Sci. Instrum. 79, 113104 (2008). 9 J. J. MacFarlane, J. Quant. Spectrosc. Radiat. Transfer 81, 287 (2003).

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Intense high repetition rate Mo Kα x-ray source generated from laser solid interaction for imaging application.

We report an efficient Mo Kα x-ray source produced by interaction of femtosecond Ti: sapphire laser pulses with a solid Molybdenum target working at 1...
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